(Re-uploaded to fix minor issues from previous attempt.)
A compilation CD of 23 various anime OPs (and 1 ED technically) from 1968 to 1972. Released in 1990 as part of a big 6 volume box set which was basically a treasure trove for any Showa-era pop culture enthusiast. Featuring stuff from TV, anime, commercials and even radio personalities of the day. Only volumes 1 and 2 specifically are about anime, and I will eventually track down volume 1 for completion's sake.
Disclaimer : A few of the tracks are cheats and are using audio not taken from an original master, so they will sound tinny and grainy. The rest are good.
Since this particular album is not in any databases I had to fill in all the artist and series info by hand, so forgive me if I got something wrong.
Enjoy, and please seed.
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HAYAKU-tan